About half of Donald's papers consist of diaries giving brief daily records of his professional and sometimes personal activities from 1918 to 1981. The remaining files fall into two series. Essays and addresses, 1919-1962, largely on economic aspects of the chemical industry, were addressed to professional organizations and commercial bodies such as the Engineering Institute of Canada, the Canadian Chemical Association, the Canadian Chamber of Commerce, and the Industrial Development Board of Manitoba. More informal speeches include a radio talk on jobs in the chemical industry, 1938. Personal materials comprise some family, legal and investment records, 1940-1952, and undergraduate essay on medieval universities, 1910, correspondence related to an annuity fund set up by Donald for Jessie Henderson, secretary and librarian of McGill's Chemistry Department (1946-1961), and a file of press releases and congratulatory letters on Donald's receipt of the Chemical Industry Medal, 1952-1953.

Collection consists of photograph albums and publications from Jean Drapeau's library related to significant events that occurred during his mandates as mayor of Montreal (1954 to 1957 and 1960 to 1986). Photograph albums, brochures, and publications represent Expo 67 and its reiteration, Man and his World (Terre des Hommes), which ran from 1968 to 1986. The 1976 Montreal Olympic Games are documented in programmes and photograph albums. The collection also includes records of Drapeau's political life, including transcripts of his speeches from 1955-1957, photograph albums related to his municipal political party, the Civic Party of Montreal (Parti civique de Montréal), and presentation copies of books.